C. Castiglioni et al., MOLECULAR FIRST HYPERPOLARIZABILITY OF PUSH-PULL POLYENES - RELATIONSHIP BETWEEN ELECTRONIC AND VIBRATIONAL CONTRIBUTION BY A 2-STATE MODEL- REPLY, Physical review. B, Condensed matter, 56(4), 1997, pp. 2275-2276
In this paper we justify the approximations we have used in the treatm
ent of Raman intensities in the paper being commented on [C. Castiglio
ni, M. Del Zoppo, and G. Zerbi, Phys. Rev. B 53, 13 319 (1996)]. This
discussion gives further support to the applicability of the expressio
ns presented by Castiglioni, Del Zoppo, and Zerbi [Phys. Rev. B 53, 13
319 (1996)], which relate electronic and vibrational first hyperpolar
izability of push-pull polyenes.