Sr. Biegalski et al., HIGH BROMINE AEROSOL CONCENTRATIONS NEAR LAKE HURON FROM LONG-RANGE TRANSPORT FROM THE ARCTIC DURING POLAR SUNRISE, JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 102(D19), 1997, pp. 23337-23343
Aerosol samples were collected at the Burnt Island sampling station in
the northern part of Lake Huron, Canada. These samples were analyzed
for trace elements via neutron activation analysis and aerosol concent
rations were determined for the time period from 1992 through 1994. Th
e seasonal trends of these aerosols were investigated and the results
for bromine indicated seasonal highs in the month of March. This was d
ifferent from the trend displayed by sodium whose peak was not as pron
ounced. Sodium was an indicator of the salt component of the aerosol t
hat Br was associated with at this site. Wind trajectory end-point ana
lysis was utilized to show that the high Br aerosol concentrations ori
ginate from the Arctic where Br aerosols have seasonal highs in the sp
ring due to the photo-induced production of particulate Br. This resea
rch shows that the highest levels of the Br aerosol in the rural north
Lake Huron area originate from the production of Br in the Arctic.