G. Irmer et al., LIGHT-SCATTERING BY A MULTICOMPONENT PLASMA COUPLED WITH LONGITUDINAL-OPTICAL PHONONS - RAMAN-SPECTRA OF P-TYPE GAAS-ZN, Physical review. B, Condensed matter, 56(15), 1997, pp. 9524-9538
The LO-phonon-hole-plasmon coupling is investigated for p-type III-V s
emiconductors. Due to a large carrier damping, only one coupled LO-pho
non-plasmon mode (CPPM) appears. Expressions for the theoretical Raman
scattering efficiency of a multicomponent plasma are derived in the r
andom phase approximation. They take into account wave-vector-dependen
t intraband transitions within the heavy-and light-hole bands as well
as interband transitions between them. Finite lifetime effects were in
cluded in a generalized Mermin approximation. The theoretical band sha
pes of the CPPM at different temperatures are compared with Raman meas
urements of Zn-doped p-type GaAs in the hole concentration range p=10(
17)-10(20) cm(-3). At low temperatures the contribution of the interba
nd transitions cannot be neglected in the frequency range of the CPPM,
resulting in a mode broadening. Agreement between the theoretical ban
d shapes and the Raman spectra is obtained without any fit parameter i
f the hole concentration p and the mobility mu are derived from the me
asured Hall values p(H) and mu(H) evaluated on the basis of a two-band
model of the conductivity. Raman measurements of the CPPM in Zn-doped
p-type GaP show a different temperature dependence, which is explaine
d by the different ratio of the light-to the heavy-hole effective mass
on the interband transitions.