CATALYTIC PARTIAL OXIDATION OF METHANE IN A NOVEL HEAT-INTEGRATED WALL REACTOR

Citation
T. Ioannides et Xe. Verykios, CATALYTIC PARTIAL OXIDATION OF METHANE IN A NOVEL HEAT-INTEGRATED WALL REACTOR, Catalysis letters, 47(3-4), 1997, pp. 183-188
Citations number
15
Categorie Soggetti
Chemistry Physical
Journal title
ISSN journal
1011372X
Volume
47
Issue
3-4
Year of publication
1997
Pages
183 - 188
Database
ISI
SICI code
1011-372X(1997)47:3-4<183:CPOOMI>2.0.ZU;2-7
Abstract
A novel reactor has been developed and applied in the reaction of part ial oxidation of methane to synthesis gas. The reactor consists of a c eramic tube in the inner and outer surface of which a metal catalyst f ilm is deposited. The CH4/O-2 feed enters into the tube and a large fr action of the heat generated on the wall by methane combustion is tran sported across the tube wall towards the outer catalyst film, where th e endothermic reforming reactions take place. In this way, the tempera ture in the combustion zone is controlled and hot spots are significan tly reduced in magnitude. Initial results presented in this work demon strate the feasibility of the concept.