Jc. Gottifredi et al., DIFFUSION AND REACTION INSIDE A CATALYST PELLET FOR A PARALLEL CONSECUTIVE REACTION SCHEME, Chemical Engineering Science, 49(15), 1994, pp. 2399-2403
An analytical solution is presented for the concentration profiles ins
ide a catalyst particle with uniform activity for a parallel-consecuti
ve reaction scheme containing a reversible step and in which the react
ions are all of the first order. An accurate approximate solution for
the surface fluxes was developed for the case of non-uniform activity.
The effects of the degree of reversibility of the first step of the c
onsecutive chain and of the ratio of the surface concentrations of the
intermediate and feed component are illustrated. The influence of a n
on uniform catalyst activity is shown to be important, particularly in
the mixed control regime.