DIFFUSION AND REACTION INSIDE A CATALYST PELLET FOR A PARALLEL CONSECUTIVE REACTION SCHEME

Citation
Jc. Gottifredi et al., DIFFUSION AND REACTION INSIDE A CATALYST PELLET FOR A PARALLEL CONSECUTIVE REACTION SCHEME, Chemical Engineering Science, 49(15), 1994, pp. 2399-2403
Citations number
11
Categorie Soggetti
Engineering, Chemical
ISSN journal
00092509
Volume
49
Issue
15
Year of publication
1994
Pages
2399 - 2403
Database
ISI
SICI code
0009-2509(1994)49:15<2399:DARIAC>2.0.ZU;2-B
Abstract
An analytical solution is presented for the concentration profiles ins ide a catalyst particle with uniform activity for a parallel-consecuti ve reaction scheme containing a reversible step and in which the react ions are all of the first order. An accurate approximate solution for the surface fluxes was developed for the case of non-uniform activity. The effects of the degree of reversibility of the first step of the c onsecutive chain and of the ratio of the surface concentrations of the intermediate and feed component are illustrated. The influence of a n on uniform catalyst activity is shown to be important, particularly in the mixed control regime.