We report the detection of carbon monoxide in the atmosphere of the br
own dwarf Gliese 229B in spectra obtained at wavelengths near 4.7 mu m
. The spectrum is consistent with mole fractions of CO of more than 50
parts per million (ppm), much higher than expected for gas in thermoc
hemical equilibrium at the temperature of the atmosphere we observe. A
s in Jupiter, mixing in the upper atmosphere of Gl 229B may prevent eq
uilibrium between CO and CH4 at low temperatures. The average flux fro
m 4.55 to 5.10 mu m in Gl 229B is measured to be 3.6 +/- 0.2 mJy, lowe
r than previous broadband measurements.