DIRECT OBSERVATION OF SPECTRAL SUBSTRUCTURE IN THE Q(Y)-ABSORPTION BAND OF LIGHT-HARVESTING COMPLEX-II BY NONLINEAR POLARIZATION SPECTROSCOPY IN THE FREQUENCY-DOMAIN AT LOW-TEMPERATURE
A. Schubert et al., DIRECT OBSERVATION OF SPECTRAL SUBSTRUCTURE IN THE Q(Y)-ABSORPTION BAND OF LIGHT-HARVESTING COMPLEX-II BY NONLINEAR POLARIZATION SPECTROSCOPY IN THE FREQUENCY-DOMAIN AT LOW-TEMPERATURE, Biochimica et biophysica acta. Bioenergetics, 1321(3), 1997, pp. 195-199
The unique high spectral resolution resulting from application of nonl
inear polarisation spectroscopy in the frequency domain at 77 K direct
ly reveals 6 subbands (at 649, 657, 667, 672, 675 and 679 nm) in the c
hlorophyll a/b Q(y)-region of trimeric light-harvesting complex II. A
shortening (from about 90 to 35 fs) of the corresponding dephasing tim
es towards the 'blue' edge of the Q(y)-band was observed. (C) 1997 Els
evier Science B.V.