C. Liousse et al., REMOTE-SENSING OF CARBONACEOUS AEROSOL PRODUCTION BY AFRICAN SAVANNA BIOMASS BURNING, JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 102(D5), 1997, pp. 5895-5911
We present an estimate of the yearly flux of total and black carbon ae
rosols emitted by savanna biomass burning in Africa from satellite dat
a and ground-based measurements. Smoke plumes are identified using vis
ible, near-infrared, and thermal infrared derived information. In the
savanna region of our study, these structures could either decrease or
increase the visible albedo of advanced very high resolution radiomet
er (AVHRR). It is hypothesized that variations of chemical composition
and particulate size distribution may create such differences. The 5S
model [Tanre et al., 1990] is used to simulate radiative transfer thr
ough smoke plumes and background atmosphere. The overall uncertainty o
f the derived aerosol optical depth (tau(a)) is 75% and mainly due to
the choice in particulate composition and size distribution aerosol. I
mpact of the aerosol mixture (internal versus external mixture) has be
en also tested. For smoke plumes a typical value of tau(a) (at 0.55 mu
m) is 0.5, and 0.1 for the background atmosphere. Specific extinction
cross sections are calculated using Mie theory applied to different r
epresentative aerosol models, allowing the retrieval of aerosol column
ar concentrations from aerosol optical depth values and integrated aer
osol mass loadings in fire plumes. The overall uncertainty on the dete
rmination of aerosol load is estimated to be lower than a factor of 5.
The atmospheric carbonaceous aerosol flux from savanna burning in Afr
ica was estimated to be 6.5 Tg C yr(-1), which compares with that obta
ined from emission factor on-site measurements (13 +/- 5 Tg C yr(-1)).