Jf. Sisler et Wc. Malm, CHARACTERISTICS OF WINTER AND SUMMER AEROSOL MASS AND LIGHT EXTINCTION ON THE COLORADO PLATEAU, Journal of the Air & Waste Management Association [1995], 47(3), 1997, pp. 317-330
This paper focuses on the spatial variability of fine mass and extinct
ion budgets taking data from the winter and summer months of 1992. The
study area included southern California, southern Nevada, southern Ut
ah, Arizona, and parts of New Mexico. Two types of monitoring sites we
re operated: intensive and secondary or satellite. At the intensive si
tes, all major aerosol species were measured as well as extinction or
scattering. At the satellite sites, trace elements including sulfur an
d hydrogen, absorption, and gravimetric fine mass were measured. Where
all aerosol species are measured, the spatial variability of extincti
on budgets is examined assuming an externally mixed aerosol. At the sa
tellite sites, an approximated fine mass budget is derived and the var
iability of these budgets in space and time are examined. This effort
was part of a study called Project MOHAVE (Measurement of Haze and Vis
ual Effects) carried out with the principal objective of understanding
the relative contribution of regional and local sources to visibility
impairment on the Colorado Plateau and specifically, the Grand Canyon
. Generally, the contribution of sulfates, organics, and absorption to
extinction are about equal at 20-30% with the coarse mass fraction be
ing about 10-20%. The one exception is in southern California where th
e nitrate contribution is significant. Furthermore, the nitrate contri
bution tends to be higher in the winter than summer. During the summer
, concentration gradients tend to be spread out across the study area,
while during the winter months, variability in concentration and budg
ets tends to occur on a smaller scale.