L. Museur et al., A VERY CONVENIENT SETUP TO GENERATE INTENSE VUV COHERENT-LIGHT AT 125NM WITH USE OF NONLINEAR EFFECTS IN MERCURY-VAPOR AT ROOM-TEMPERATURE, IEEE journal of selected topics in quantum electronics, 1(3), 1995, pp. 900-907
Using only one dye laser, efficient generation of VUV radiation (10(13
) photons/pulse) is demonstrated at 125.140 nm and 125.053 nm by four-
wave sum-frequency mixing in a room-temperature mercury vapor. The emi
ssion at 125.053 nm, which is out of two-photon resonance, but near th
ree-photon resonance, has been observed for the first time and is care
fully analyzed. In particular, numerical calculations have been carrie
d out for Gaussian pump beams, taking into account absorption of VUV p
hotons and optical Kerr effect. The results of the calculations reprod
uce the VUV emission lineshape and power saturation effects measured i
n the experiment.