M. Poirier et al., MAGNETOELASTIC COUPLING AND ORDER-PARAMETER IN THE SPIN-PEIERLS SYSTEM CUGEO3, Physical review. B, Condensed matter, 52(22), 1995, pp. 16058-16065
The anomalous elastic character of the dimerization axis in the spin-P
eierls system CuGeO3 is established above and below the transition tem
perature T-sp by studying, in a magnetic field, the propagation of lon
gitudinal ultrasonic waves along the three crystalline directions. At
high temperatures an important anomaly on the elastic constant C-33 is
identified and discussed in relation with lattice fluctuations recent
ly observed below 100 K in an electron diffraction experiment and attr
ibuted to vibrations of CuO2 ribbons along the chain. Stiffening anoma
lies are observed along the three crystalline directions below T-sp; a
softening of the velocity is seen only along the chain axis above the
transition. The temperature acid magnetic-field dependences of these
anomalies are studied with a Landau free-energy model for the magnetoe
lastic coupling which gives access to the order parameter, the magneti
c gap.