An experimental study of the structure of round buoyant turbulent plum
es was carried out, emphasizing conditions in the fully developed (sel
f-preserving) portion of the flow. Plume conditions were simulated usi
ng dense gas sources (carbon dioxide and sulfur hexafluoride) in a sti
ll air environment. Mean and fluctuating mixture fraction properties w
ere measured using single-and two-point laser-induced iodine fluoresce
nce. The present measurements extended farther from the source (up to
151 source diameters) than most earlier measurements (up to 62 source
diameters) and indicated that self-preserving turbulent plumes are nar
rower, with larger mean and fluctuating mixture fractions (when approp
riately scaled) near the axis, than previously thought. Other mixture
fraction measurements reported include probability density functions,
temporal power spectra, radial spatial correlations and temporal and s
patial integral scales.