H. Vanmalderen et al., CHEMICAL CHARACTERIZATION OF INDIVIDUAL AEROSOL-PARTICLES IN CENTRAL SIBERIA, Environmental science & technology, 30(1), 1996, pp. 312-321
In order to characterize the Siberian aerosol, more than 120 samples f
or single-particle analysis have been collected simultaneously at two
sampling stations in central Siberia in 1 month's time during February
and August 1992. For each sample, 400 particles have been analyzed wi
th automated electron probe X-ray microanalysis. Hierarchical cluster
analysis allowed us to identify nine major particle types. The differe
nces in aerosol composition were found to be bigger between the winter
and summer campaigns than between the two sampling locations. Nonhier
archical cluster analysis combined with 36-h backward air mass traject
ories permitted us to compare the abundances for the major particle ty
pes for four different source sectors. Results showed significant, tho
ugh not enormous, differences. Source identification by principal fact
or analysis allowed the identification of several sources for the Sibe
rian aerosol. Our results provide ample evidence for a long-suspected
contribution to Arctic pollution by industrial complexes in the former
Soviet Union.