V. Vohra et Rh. Heist, THE FLOW DIFFUSION NUCLEATION CHAMBER - A QUANTITATIVE TOOL FOR NUCLEATION RESEARCH, The Journal of chemical physics, 104(1), 1996, pp. 382-395
We have developed a flow diffusion nucleation chamber designed to quan
titatively investigate the nucleation of vapors. The design and operat
ional characteristics of the nucleation chamber are presented and disc
ussed. Critical supersaturation data obtained with this nucleation cha
mber are compared to literature data obtained using a thermal diffusio
n cloud chamber. The flow nucleation chamber results accurately reprod
uce the diffusion cloud chamber data. Results of preliminary measureme
nts of nucleation at ambient pressure in the presence of different bac
kground gases are presented. These data suggest that the nature of the
background gas may influence nucleation at ambient pressure. These da
ta, while still of a preliminary nature, are consistent with data alre
ady published obtained at elevated pressures using a specially designe
d high pressure cloud chamber also in our laboratory. (C) 1996 America
n Institute of Physics.