2-STEP COULOMB EXPLOSIONS OF DIATOMS IN INTENSE LASER FIELDS

Citation
S. Chelkowski et Ad. Bandrauk, 2-STEP COULOMB EXPLOSIONS OF DIATOMS IN INTENSE LASER FIELDS, Journal of physics. B, Atomic molecular and optical physics, 28(23), 1995, pp. 723-731
Citations number
15
Categorie Soggetti
Physics, Atomic, Molecular & Chemical",Optics
ISSN journal
09534075
Volume
28
Issue
23
Year of publication
1995
Pages
723 - 731
Database
ISI
SICI code
0953-4075(1995)28:23<723:2CEODI>2.0.ZU;2-M
Abstract
A two-step model of Coulomb explosions of diatoms in intense laser fie lds is presented. In this model the molecule loses several electrons w hen the atoms are at the equilibrium internuclear distance and then fa st Coulomb explosions occur until the products reach a critical distan ce R(c) congruent to 9 Bohr, at which several additional electrons are lost due to a recently discovered maxima of ionization rates occurrin g at R = R(c). Then the subsequent Coulomb explosion for the higher-ch arged ions takes place. The total combined Coulomb explosion energy ag rees well with experimental results, showing striking regularities. Th e origin and intensity dependence of unexpectedly high ionization rate s of dissociating nuclei at preferential, large internuclear distances R = R(c) is also discussed and an analytic expression for R(c) is der ived.