Jl. Jaffrezo et Ci. Davidson, THE DYE-3 GAS AND AEROSOL SAMPLING PROGRAM (DGASP) - AN OVERVIEW, Atmospheric environment. Part A, General topics, 27(17-18), 1993, pp. 2703-2707
DGASP was designed as an international effort to study the processes i
nfluencing chemical species that eventually reach the deep ice in the
south of Greenland. These processes include long-range atmospheric tra
nsport, wet and dry deposition to the snow surface, and changes during
aging of the snow. The program took place during August 1988-July 198
9. Experimental work included sampling of aerosols and gases, collecti
on of fresh and older surface snow, and sampling of snowpits. The vari
ous samples were analysed for chemical species that are tracers of spe
cific source categories. Results of the program show that the southern
Greenland Ice Sheet experiences very different airborne concentration
patterns than sea-level arctic sites. Concentrations of SO42-, trace
metals, and other species are episodic and peak in April, unlike the c
onsistently high concentrations during January-April seen at lower ele
vations. Source regions influencing Dye 3 are variable, and include No
rth America, western Europe, and the Arctic Basin. The last region is
particularly important, as it may contain relatively high concentratio
ns of chemical constituents from eastern Europe and western Asia that
eventually reach Dye 3. The seasonal variations in airborne concentrat
ions are generally also reflected in fresh snow. Similarly, these patt
erns are seen in snowpits, although some modifications to the glacial
record are apparent. Other information on the extent of riming, aeroso
l/gas partitioning, and aerosol size distributions demonstrate the com
plexity of air-snow transfer processes, and illustrate the need for fu
rther research.