C. Lombardi et A. Mazzola, PLUTONIUM BURNING IN PRESSURIZED-WATER REACTORS VIA NONFERTILE MATRICES, Nuclear science and engineering, 122(2), 1996, pp. 229-239
The plutonium that comes from dismantled warheads and that is already
stockpiled from commercial fuel reprocessing has raised many proposals
for its burning in a safe and economical manner. The utilization is e
xamined of current pressurized water reactors (PWRs) that are partiall
y fed with a nonfertile oxide-type fuel, while the rest of the core is
still fed with standard U-235-enriched fuel. The unconventional fuel
consists of PuO2 diluted in an inert matrix, which should be highly ra
diation resistant, scarcely neutron absorbent, and chemically stable a
nd which allows the final disposal of the discharged fuel without any
treatment. Commercial PWRs operating in a once-through cycle scheme ca
n transmute 97 to 99% of Pu-239 and 71 to 84% of total initially loade
d reactor- and weapons-grade plutonium, respectively. The remnant plut
onium is in a proliferation-resistant condition. The high initial reac
tivity of the plutonium-bearing rods causes a high initial rod power p
eak and continuously decreasing power generation in these rods during
the irradiation. A less pronounced rod power peak in UO2 rods at end o
f life has to be addressed. The reactivity coefficients are, in absolu
te terms, slightly lower than the standard UO2 fuel ones.