Mbl. Santos et al., MICELLAR FLUCTUATIONS IN A CALAMITIC NEMATIC PHASE OF A LYOTROPIC LIQUID-CRYSTAL STUDIED BY PHOTON-CORRELATION, Liquid crystals, 16(2), 1994, pp. 287-298
Using a Rayleigh scattering light beating technique, we have made new
measurements on the slow polarized fluctuations, previously identified
as being of micellar origin, for a lyotropic system consisting of K-l
aurate, decanol, D2O and presenting only the uniaxial calamitic nemati
c (N(C)) phase (from among the three known nematic types: uniaxial dis
k-like (N(D)), Calamitic (N(C)) and biaxial (N(B)) phases). An elabora
ted analysis of these data is made in order to clarify the relationshi
p between the light scattering signals coming from the micellar fluctu
ations and those from (classical) orientational fluctuations. The main
conclusions of this analysis are that the micellar mode is independen
t of the temperature and wavevector, and that its relaxation frequency
is substantially lower than that found previously for the same lyotro
pic components, but presenting the biaxial nematic phase. Finally, som
e considerations are made of the possible relationships between the mi
cellar fluctuations and the structural properties of lyotropic nematic
s.