R. Caporali et al., SURFACE BRILLOUIN-SCATTERING SPECTROSCOPY OF MEDIA WITH NONUNIFORM ACOUSTOOPTIC PROPERTIES, Physical review. B, Condensed matter, 53(7), 1996, pp. 4133-4141
We present a theoretical tool to compute the Brillouin-scattering cros
s section for shear horizontal (SH) surface phonons in an inhomogeneou
s medium with any type of depth profiles of elastic, dielectric, and e
lasto-optic properties. The acoustic eigenmodes are found by means of
numerical solution of a self-adjoint Liouville equation with the bound
ary conditions of a finite slab. Both discrete and continuous phonon s
pectra are studied. The layer projected phonon density of states for t
he SH polarization is used to analyze the surface character of the mod
es. Also, the transmitted (zeroth-order) electromagnetic field and the
reflection coefficient are obtained numerically solving Maxwell's equ
ations. The scattered field is computed (in a way similar to that of t
he zeroth-order field) by first-order perturbation theory as a result
of the smallness of the phonon excitations. The backscattering p-s Bri
llouin spectrum is obtained by summing the scattering intensity from i
ndividual acoustic modes over the density of phonon states at a generi
c incidence angle. As an example, we present the case of a Si/SiO2, bi
layer on a Si(001) substrate with sharp or smooth interfaces between s
ilicon and silica. We think the method is promising in view of the app
lication of surface Brillouin-scattering spectroscopy to real imperfec
t materials.