Thermal-expansion measurements of (FeF2)n(ZnF2)m magnetic/nonmagnetic
superlattices high-resolution x-ray diffraction have been made through
out the antiferromagnetic phase-transition region. Using the proportio
nality of the magnetically induced thermal expansion to the magnetic s
pecific heat, the experimental results are compared with detailed Mont
e Carlo simulations. Both the experimental and Monte Carlo data are an
alyzed in terms of finite-size scaling theory. From this combined anal
ysis, we are able to show that the observed shifts in the phase-transi
tion temperature with respect to bulk FeF2 arise from three-dimensiona
l to two-dimensional Ising-model crossover behavior. To our knowledge,
this is the first time that dimensional crossover in a real Ising-lik
e magnetic system has been experimentally observed.