Thus far, a good Kerr hysteresis loop has been obtained only for thick
ness ratios of Co to Pt lower than 0.6 in Co/Pt multilayers. It has be
en found in this study that perfect squareness can be obtained for ult
rathin films even with a high thickness ratio of t(Co)/t(Pt) = 1. This
is caused by diminished magnetostatic energy. Furthermore, layer-modu
lated structures were investigated in order to increase the Kerr rotat
ion angle. The Co/Pt multilayers were prepared by two-source rf-magnet
ron sputtering. Co/Pt multilayers with perfect squareness were deposit
ed with a Pt interlayer, which resulted in excellent magneto-optical p
roperties. In particular, the Kerr rotation angle measured from the gl
ass-substrate side showed a very large value, 0.73 degrees. This Kerr
enhancement is due to optical interference and multiple reflection. On
the other hand, another interesting phenomenon was also obtained. Ker
r hysteresis showed characteristic stepwise hysteresis loops when the
interlayer Pt thickness was increased. Such layer-modulated multilayer
s have potentiality for high-density magneto-optical recording.