H. Ozkaynak et al., PERSONAL EXPOSURE TO AIRBORNE PARTICLES AND METALS - RESULTS FROM THEPARTICLE TEAM STUDY IN RIVERSIDE, CALIFORNIA, Journal of exposure analysis and environmental epidemiology, 6(1), 1996, pp. 57-78
The PTEAM Study was the first large-scale probability-based study of p
ersonal exposure to particles. Sponsored by the U.S. Environmental Pro
tection Agency (EPA) and the Air Resources Board of California, it was
carried out by the Research Triangle Institute (RTI) and the Harvard
University School of Public Health (HSPH). HSPH designed and construct
ed a 4-lpm, battery-operated personal monitor for inhalable particles
(PM(10)) that could be wont comfortably for up to 14 hours by persons
from 10 to 70 years old. The monitor was worn for two consecutive 12-h
our periods (day and night) during the fall of 1990 by 178 participant
s representing 139,000 nonsmoking residents of Riverside, California.
Nearly identical monitors were employed to collect concurrent indoor a
nd outdoor samples. The monitors were equipped with a different sampli
ng nozzle to collect fine particles (PM(2.5)). Population-weighted day
time personal PM(10) exposures averaged 150 +/- 9 (SE) mu g/m(3), comp
ared to concurrent indoor and outdoor concentrations of 95 +/- 6 mu g/
m(3). This suggested the existence of excess mass near the person, a '
'personal cloud'' that appeared related to personal activities. Fourte
en of 15 prevalent elements also were elevated in the personal samples
. The two major indoor sources of indoor particles were smoking and co
oking; even in these homes, however, more than half of the indoor part
icles came from outdoors, and a substantial portion of the indoor part
icles were of undetermined indoor origin.Outdoor concentrations near t
he homes were well correlated with outdoor concentrations at the centr
al site, supporting the idea of using the central site as an indicator
of ambient concentrations over a wider area. Indoor concentrations we
re only weakly correlated with outdoor concentrations, however, and pe
rsonal exposures were even more poorly correlated with outdoor concent
rations. Elemental profiles were obtained for environmental tobacco sm
oke (ETS) (major contributions from potassium and chlorine) and cookin
g emissions (aluminum, iron, calcium, and chlorine). These profiles ca
n be used in future source apportionment studies.