B. Wuyts et al., RESISTIVITY AND HALL-EFFECT OF METALLIC OXYGEN-DEFICIENT YBA2CU3OX FILMS IN THE NORMAL-STATE, Physical review. B, Condensed matter, 53(14), 1996, pp. 9418-9432
We present a systematic study of normal-state transport properties in
a series of c-axis-oriented YBa2Cu3Ox (YBCO) epitaxial thin films and
YBa2CU3O7/PrBa2Cu3O7 (YBCO/PrBCO) superlattices. The hole doping level
in the YBCO films is varied from the optimum-doped metallic down to t
he underdoped insulating regime by changes in the oxygen content x. We
find that the magnitude of the resistivity rho and Hall coefficient R
(H) increases monotonically with decreasing x and that their respectiv
e temperature dependences undergo marked changes. The R(H)(T) behavior
is reminescent of the Hall effect behavior in heavy fermion metals, t
aking into account a difference in temperature by a factor of LOG. The
Hall angle Cot theta(H) = rho/R(H)B shows a qundraticlike temperature
dependence, with systematic deviations at high and low doping levels.
Transport measurements in YBCO/PrBCO superlattices, with the YBCO lay
ers in the two-dimensional regime, indicate that the deviations of a T
-2 dependence of the Hall angle art intrinsic and not related to the d
imensionality of the system. A method of analyzing the transport data
is presented, revealing a striking scaling behavior of the respective
properties. A comparison with reported transport data in the literatur
e suggests that the observed scaling behavior may be universal for und
erdoped cuprates. Furthermore, we show that reported NMR Knight shift
data for oxygen-deficient YBCO samples can also be mapped on a single
scaling curve, by using the same scaling parameter derived from our tr
ansport measurements. This finding strongly indicates that the dominan
t scattering mechanism in these materials is of magnetic origin. Going
one step further, we present a qualitative analysis of the conductivi
ty under the assumption that we may use the expression for a two-dimen
sional quantum liquid and that the inelastic scattering length may be
replaced by the magnetic correlation length xi(T). Expressions for the
latter are taken from reported calculations for undoped and doped cup
rates. A good qualitative agreement is obtained between the calculated
and experimentally observed temperature-dependent conductivity.