MAGNETIC RAMAN-SCATTERING IN UNDOPED AND DOPED ANTIFERROMAGNETS

Citation
M. Pressl et al., MAGNETIC RAMAN-SCATTERING IN UNDOPED AND DOPED ANTIFERROMAGNETS, Journal of Raman spectroscopy, 27(3-4), 1996, pp. 343-349
Citations number
35
Categorie Soggetti
Spectroscopy
ISSN journal
03770486
Volume
27
Issue
3-4
Year of publication
1996
Pages
343 - 349
Database
ISI
SICI code
0377-0486(1996)27:3-4<343:MRIUAD>2.0.ZU;2-E
Abstract
Magnetic Raman scattering of doped and undoped high-T-c (HTc) cuprates is presented in comparison with the conventional antiferromagnet NiO, In both classes of materials the strong magnetic Raman response is ca used by a Me-O superexchange mechanism, The difference in the absolute Raman cross-sections of 90 x 10(-5) sr(-1) cm(-1) (YBa2Cu3O6.3) and 1 .6 x 10(-5) sr(-1) cm(-1) (NiO) is explained by the different strength s of the exchange energies. The magnetic scattering signal of NiO is e xplainable by the pure Heisenberg model, whereas the zone edge magnons of the HTc cuprates show additional damping due to magnon phonon inte raction, On doping, the damping of the zone-edge magnons increases by a factor of 4 more than the decrease of magnon energy, This is charact eristic of the interaction of the spin system with the charge carriers , The absolute Raman cross-section is reduced owing to the interruptio n of antiferromagnetic spin correlations on doping.