We have investigated ultrathin FexNi1-x films grown epitaxially on Cu(
100) with different stochiometry. With the surface magneto-optic Kerr
effect (SMOKE) we measured the variation of the Curie temperature T-C
as a function of the film thickness n in monolayers (ML). Using the re
sults of our previous investigations on finite-size scaling (Huang et
al.), we are able to extrapolate the value T-C(infinity) for samples w
ith different Fe content. In particular, alloy films with Fe concentra
tions close to 65% remain ferromagnetic. This is in contrast to bulk F
e65Ni35, which shows a collapse of long range order, which is the so-c
alled invar effect associated with a fcc to bcc structural transition.
Growing these alloy films on a Cu(100) substrate forces them to adapt
the Cu lattice spacing, thereby suppressing the structural relaxation
. (C) 1996 American Institute of Physics.