In previous work we reported that the magnetoresistance of Fe/Cr multi
layers can be increased by annealing the films at moderate temperature
s, which increases the spin-dependent scattering of the conduction ele
ctrons. Here we present Mossbauer data that demonstrate that the struc
tural effect of annealing is to promote Cr interdiffusion into the bul
k of the iron layers rather than short scale intermixing at the interf
aces. We have also investigated the effect of increasing the asymmetri
c scattering by adding chromium to the iron in Fe/Cr multilayers. The
additional Cr was either alloyed with the Fe in compositions ranging f
rom 1.5% to 50% Cr in Fe, or concentrated into 1 or 2 Angstrom layers
embedded at various positions in the Fe. We report enhanced room-tempe
rature magnetoresistance of up to 11.4% in sputter-deposited Fe/Cr mul
tilayers when the Fe layers are doped with 20% Cr. The maximum magneto
resistance observed for samples with embedded Cr layers was 10.5%. In
comparison, the magnetoresistance was 7.5% in a similar, undoped sampl
e. (C) 1996 American Institute of Physics.