Fe. Kruis et L. Falk, MIXING AND REACTION IN A TUBULAR JET REACTOR - A COMPARISON OF EXPERIMENTS WITH A MODEL-BASED ON A PRESCRIBED PDF, Chemical Engineering Science, 51(10), 1996, pp. 2439-2448
The simulation of chemical reactions in a turbulent fluid is very impo
rtant for industrial applications. In particular, models which demand
only moderate computational times while still taking into account the
inhomogeneity of the reactor are of practical interest. An approach is
presented here which applies a simulation of the turbulent now field
in describing the transport production and dissipation of a non-reacti
ve tracer. Two modelling approaches (the turbulent mixer model of Bald
yga and the spectral relaxation model of Fox) are compared with experi
mental data of a laboratory tubular jet reactor. The turbulent flow fi
eld was obtained from a computational fluid dynamics code using the k-
epsilon model. The closure approximation of Baldyga, which is based on
a prescribed form of the probability density function is applied in m
odelling chemical reactions. Simulations were performed for a series-p
arallel reaction.