L. Zanderighi et al., EVALUATION OF THE PERFORMANCE OF MULTISTAGE MEMBRANE SEPARATION CASCADES, Separation science and technology, 31(9), 1996, pp. 1291-1308
The minimization of the work consumption in a multistage membrane sepa
ration cascade operating in isoenthalpic conditions was investigated w
ith regard to the splitting factor of each stage, for the assigned val
ues of the number of stages, the retentate and permeate pressures, and
the flow pattern. The mathematical model of the membrane separation c
ascade is presented, and five possible different flow patterns togethe
r with system variance are discussed. Under isoenthalpic conditions th
e work needs are due to the compression of the permeated stream, and t
he work losses to the generation of entropy on the mixing of recycled
streams. A three-component mixture (NH3, H-2, N-2) and a polyethylene
membrane were used as the standard testing system; the results of the
optimization for three, five, seven, or nine stages cascades, using as
the initial splitting factor values 0.5, 1.0, and 1.5 for all stages,
are discussed. Increasing the number of stages increases the membrane
surface area and the total work consumption owing to the increase in
recycled stream flow. In the case under examination, both the efficien
cy index and the specific efficiency decrease for cascades of more tha
n five stages. Therefore membrane staging seems to be unattractive fro
m the point of view of both capital investment and operating costs, at
least for more than a certain number of stages, depending on the spec
ific problem.