Mixtures of FN3, I-2, HF, and He were shock heated by reflection of an
Ma similar to 2 incident wave to generate peak metastable NF concent
rations > 10(16)/cm(3). Time profiles of the NF(a), NF(b), I-2, and I
concentrations were optically measured and fit to a chemical kinetics
and gas dynamic model of the reaction process. Approximately six NF
molecules were consumed per I-2 molecule dissociated, and energy trans
fer from NF(a) to I was both fast and efficient. Attempts to achieve
lasing on the 1315 nm (I --> I) atomic transition were unsuccessful,
however, due to rapid E-V quenching of I by the NF species present.