S. Ten et al., FEMTOSECOND STUDY OF EXCITON TUNNELING IN (ZN,CD)SE ZNSE ASYMMETRIC DOUBLE-QUANTUM WELLS/, Physical review. B, Condensed matter, 53(19), 1996, pp. 12637-12640
We have studied, both experimentally and theoretically, exciton tunnel
ing in a (Zn,Cd)Se/ZnSe asymmetric double quantum-well structure. The
large exciton binding energy of these structures allows us to elucidat
e the role of the electron-hole interaction. Subsequent to resonant fe
mtosecond pulse excitation, we observe fast (1 ps) exciton tunneling o
ut of the narrow well, although LO-phonon scattering is forbidden for
holes in a single-particle picture. Our theoretical analysis shows, ho
wever, that tunneling of the exciton as a whole entity with the emissi
on of only one LO phonon is very slow. Instead, the exciton tunnels vi
a an indirect state in a two-step process whose efficiency is dramatic
ally enhanced by Coulomb effects.