M. Hartmann et al., NONLINEAR-OPTICAL EXCITATIONS IN FEMTOSECOND SPECTROSCOPY OF CONJUGATED POLYMERS, Journal of luminescence, 66-7(1-6), 1995, pp. 97-101
We have investigated the optical excitation of solitons and charge tra
nsfer excitons in polymer chains by solving the equations of motion fo
r the reduced density matrix and the lattice displacement simultaneous
ly in time. Electron-phonon coupling leads to polaron-exciton formatio
n which can be identified in transient pump-probe signals.