Aj. Elliot et al., TEMPERATURE-DEPENDENCE OF G-VALUE FOR AQUEOUS-SOLUTIONS IRRADIATED WITH 23 MEV H-2(-7(3+) ION-BEAMS() AND 157 MEV LI), Journal of physical chemistry, 100(21), 1996, pp. 9014-9020
The temperature (T) dependence of the g values for the radiolysis of w
ater with 23 MeV H-2(+) and 157 MeV Li-7(3+) ion beams is reported. Th
e results indicate that as the linear energy transfer characteristics
of the radiation increase, (i) d(g(e(aq)(-)))/dT decreases, (ii) d(g(H
-2)/dT increases, (iii) d(g(OH))/dT remains constant, and (iv) d(g(H2O
2))/dT is approximately constant. These observations are qualitatively
consistent with the kinetic-diffusion model of the spur/track. The g
values for 2 MeV fission neutrons have been estimated from these ion b
eam results for the temperature range 75-300 degrees C.