Four coal-tar pitches were used in conjunction with a woven carbon fib
re cloth to produce carbon/carbon (C/C) composites in order to study t
he effect of the nature of the pitch, as matrix precursor, on the prop
erties of fully-processed composites. The nature of the pitch had litt
le effect on the density, porosity, flexural modulus or inter-lamellar
shear strength of the composites. However, the flexural strength of t
he composites decreased as the quinoline insolubles (QI) content of th
e precursor pitch increased. Two structural features of the composites
also varied with the pitch QI content: the amount of granular carbon
in inter-layer positions and the mean length of bundle voids, i.e. tho
se oriented perpendicular to the cloth layers. The flexural strength c
ould be related to void parameters using an equation developed from th
e Knudsen equation. Copyright (C) 1996 Elsevier Science Ltd