M. Lepore et al., 3-PHOTON ABSORPTION-COEFFICIENTS IN ZNSE ZNS0.18SE0.82 STRAINED-LAYERSUPERLATTICES/, Nuovo cimento della Societa italiana di fisica. D, Condensed matter,atomic, molecular and chemical physics, biophysics, 18(4), 1996, pp. 465-469
We provide the first experimental determination of three-photon absorp
tion (ThPA) coefficients alpha((3)) in a quasi-bidimensional structure
. The measurements of alpha((3)) have been performed on a sample of a
ZnSe/ZnS0.18Se0.82 strained-layer superlattice at fixed excitation ene
rgies corresponding to the exciton resonances near the direct band gap
. The evidence of the ThPA process in such energy range points out the
huge enhancement of exciton non-linearities in quantum-confined syste
ms.