Using a continously tunable pulsed 20-atmosphere CO2 laser as a pump s
ource, we generated pulses of mid-infrared radiation, partly tunable i
n frequency intervals in the range between 200 and 900 cm(-1) via stim
ulated Raman scattering in gaseous ammonia. As a Raman cell we used a
multiple pass cell. We observed for (NH3)-N-14 and (NH3)-N-15 laser li
nes at 52 different frequencies with 39 lines observed for the first t
ime. Tuning ranges up to 150 GHz and peak powers of several MW were ac
hieved. The quantum efficiency reached 40 %.