Cosmic ray spallation/fusion reactions may yield astrophysically inter
esting amounts of lithium, beryllium and boron during the early evolut
ion of the Galaxy. In particular, since alpha,alpha fusion reactions c
an produce Li-6 and Li-7 whereas Be and B require CNO nuclei as spalla
tion targets, the Pop II ratios of Li to Be and/or B are vastly differ
ent from their Pop I counterparts. Current data on Pop II Be do not ex
clude the possibility that significant amounts of lithium have been pr
oduced via this mechanism. The observed increase in the Pop II abundan
ce of beryllium with increasing metallicity points to synthesis during
the early Galaxy. The boron to beryllium ratio is relatively insensit
ive to model-dependent, evolutionary uncertainties and could provide a
signature for cosmic ray nucleosynthesis during the early Galaxy.