Gf. Kventsel et Bi. Lembrikov, 2ND SOUND AND NONLINEAR-OPTICAL PHENOMENA IN SMECTIC-A LIQUID-CRYSTALS, Molecular crystals and liquid crystals science and technology. Section A, Molecular crystals and liquid crystals, 282, 1996, pp. 145-189
We investigated theoretically the nonlinear phenomena (a self-focusing
, a self-trapping, stimulated light scattering and four-wave mixing) i
n smectic A liquid crystals (SA) caused by a new physical mechanism of
cubic nonlinearity determined by the propagating mode of a layer norm
al displacement, or the so-called second sound. A nonlinear part of a
refractive index caused by a layer normal deformation which is respons
ible for a self-focusing effect, and a gain coefficient in the case of
a stimulated light scattering (SLS) on the second sound are one or tw
o orders of magnitude greater than the similar quantities for isotropi
c organic liquids. The light-induced dynamic grating of layer deformat
ions generates a high-frequency longitudinal electric field due to the
flexoelectric effect. The light-induced dynamic grating of layer norm
al displacement ultimately excites a rotational hydrodynamic how with
a considerable velocity. Using the slow varying amplitude approximatio
n we calculated the light wave and second sound wave amplitudes explic
itly for some important cases.