B. Nagels et al., GENERALIZED ANALYTICAL DESCRIPTION OF LIGHT-INDUCED DRIFT AND AN EXPERIMENTAL TEST USING C2H4, Physical review. A, 53(6), 1996, pp. 4305-4310
It is demonstrated that both standard and anomalous light-induced drif
t (LID) profiles as a function of laser frequency can be analytically
simulated using the description of LID in terms of transport mean path
s. This description allows one to directly link arbitrary LID frequenc
y profiles to derivatives of the unsaturated absorption profile. In or
der to test this approach, LID experiments have been performed on gase
ous ethylene ((CCH4)-C-13-C-12) for the rovibrational transition (7,1,
6) --> nu(7)(8,0,8) in a background of Kr, Xe, SF6, CO2, or CH3Cl. Alt
hough the observed LID frequency profiles show a large variation, they
are well simulated using this approach.