SENSITIVITY OF THE CH4 GROWTH-RATE TO CHANGES IN CH4 EMISSIONS FROM NATURAL-GAS AND COAL

Authors
Citation
Ks. Law et Eg. Nisbet, SENSITIVITY OF THE CH4 GROWTH-RATE TO CHANGES IN CH4 EMISSIONS FROM NATURAL-GAS AND COAL, JOURNAL OF GEOPHYSICAL RESEARCH-ATMOSPHERES, 101(D9), 1996, pp. 14387-14397
Citations number
51
Categorie Soggetti
Metereology & Atmospheric Sciences
Volume
101
Issue
D9
Year of publication
1996
Pages
14387 - 14397
Database
ISI
SICI code
Abstract
The observed rate of increase in atmospheric CH4 declined gradually du ring the late 1980s [Steele et al. 1992] and then fell dramatically by similar to 4 to 7 parts per billion by volume (ppbv) yr(-1) from 1991 to 1992 [Dlzcgokencky et al., 1994a]. Post-1993 the CH4 growth rate h as recovered to pre-1991 levels. In this study, we assess the sensitiv ity of the CH4 growth rate to changes in CH4 emissions from the coal a nd gas industries over the last 15 years using a global two-dimensiona l (2-D) model of the atmosphere. Emissions are estimated from availabl e production data, and in the case of natural gas, a spectrum of leaka ge rates is assumed. Changes in the former Soviet Union (FSU) have bee n assessed separately from the rest of the world (ROW). Prior to 1989, increased coal and natural gas production led to an increase in the C H4 growth rate (i.e., opposite to that which was observed). During the period 1989 to 1993 the modelled CH4 growth rate decreased by similar to 1-2 ppbv yr(-2) at northern mid-latitudes (assuming constant gas l eakage rates), showing that declining emissions, primarily in the form of natural gas from the FSU, may have contributed to the general redu ction in the CH4 growth rate from 1989 to 1991. However, this does not explain the large reduction which was observed between 1991 and 1992. A model run with FSU gas leakage rates decreasing by 1% yr(-1) from 5 % in 1990 to 2% in 1993 shows a decrease in the CH4 growth rate of sim ilar to 9-12 ppbv yr(-1) (or similar to 3-5 ppbv yr(-2)) over this per iod. This is similar in magnitude to the observed decline over the sam e period. This sensitivity study illustrates the large potential for s ignificantly lowering the growth rate of atmospheric CH4 by reducing f ossil fuel emissions from coal and, in particular, by reducing the lea kage rates from natural gas installations.