A high-intensity powder neutron diffraction study of La1.2Tb0.8CuO4 wh
ich has the tetragonal T-structure shows that the compound orders ant
iferromagnetically with a magnetic structure which can be described by
employing a magnetic propagation vector, tau = (1/2, 1/2, 0) perpendi
cular to the Cu2+ spin direction, S = (1/2, 1/2, 0) (identical to that
of La2CuO4). The staggered Cu2+ moment at 1.6 K is 0.46 (6) mu(B). Ho
wever, non-collinear spin structures are also possible. The appearance
of magnetic diffuse scattering at low temperatures is interpreted as
the signature of short range magnetic ordering of the Tb3+ ions. Essen
tially unchanged magnetic behaviour is found in the lightly-doped La1.
19Tb0.8Sr0.01CuO4 and La1.2Tb0.79Ce0.01CuO4 materials.