Various physics and computational. approaches have been developed to g
lobally characterize phenomena important for film growth by pulsed-las
er deposition of materials. These include thermal models of laser-soli
d target interactions that initiate the vapor plume, plume ionization
and heating through laser absorption beyond local thermodynamic equili
brium mechanisms, hydrodynamic and collisional descriptions of plume t
ransport, and molecular dynamics models of the interaction of plume pa
rticles with the deposition substrate.