Single-shot ablation thresholds of gold and nickel films in the thickn
ess range from 50 nm to 3.7 mu m have been measured for 8 ps, 130 ps a
nd, for comparison, 15 ns laser pulses at 248 nm. The metal films were
deposited on fused silica substrates. The topology of the ablated fil
ms was determined by an AFM. For picosecond ablation one finds an inte
resting transition range where, for the 8 ps pulses, the threshold flu
ence initially drops as the film thickness is increased, in contrast t
o the 130 ps pulses where the threshold increases with increasing film
thickness, as for ablation with the nanosecond pulses. In addition, c
omparison of the topological structure shows different behaviour for t
he Au and Ni films. The Ni films show typical material removal behavio
ur. The Au films show a melting character both for the 8 and 130 ps pu
lses. The nature of this difference is not yet clear and is the subjec
t of further investigations.