K. Kemp, LONG-TERM AEROSOL MEASUREMENTS, Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms, 109, 1996, pp. 530-535
One of the main topics addressed by the PULE community has, right from
the early days of the method, been the measurements of the elemental
content in ambient aerosols. The available time series of measurements
cover in many cases now more than one decade. Examples of the use of
these data are shown by using the results of daily measurements from 1
979 to 1994 in urban and rural areas in Denmark. The cyclic variations
as well as the trends of the concentrations are described by using i.
a. simple time-series analyses based on auto-correlation. Characterist
ic weekly and annual variations are shown for different elements. A st
rongly decreasing trend is seen for Pb, while the concentrations of ot
her heavy metals and particulate sulphur are only slightly decreasing
or almost constant, but it varies with the source areas.