V. Veniard et al., PHASE DEPENDENCE OF (N-COLOR (N-GREATER-THAN-1) IR-UV PHOTOIONIZATIONOF ATOMS WITH HIGHER HARMONICS(1)), Physical review. A, 54(1), 1996, pp. 721-728
We discuss, via a numerical calculation, the main properties of atomic
photoelectron spectra, as they would be obtained by using a radiation
pulse containing N+1 frequencies associated with a ''Dirac comb'' of
N higher harmonics together with the laser which has been used to gene
rate them. We address more precisely the physically relevant situation
in which the harmonics have much weaker intensities than the one of t
he laser. In such (N+1)-color photoionization processes, the atom can
simultaneously absorb harmonic uv photons and exchange, i.e., absorb a
nd/or emit, (via stimulated emission) laser ir photons. We have simula
ted the photoelectron spectra by numerically solving the time-dependen
t Schrodinger equation for a three-dimensional hydrogen atom in the pr
esence of the radiation pulse. Our results show that, everything else
being kept fixed, the magnitudes of the photoelectron peaks are strong
ly dependent on the difference of phase between successive harmonics.
This strong dependence results from interference effects taking place
between competing quantum paths leading to a given final state. An int
eresting feature is that these interferences involve transitions in th
e continuum states of the atom and do not depend on resonances in the
discrete spectrum. Another interesting outcome of our study is to show
that such effects should be observable with currently developed harmo
nic sources.