We observed photon-gated spectral hole burning in Pr:YAG and assigned
the hole-burning mechanism to selective photoionization of trivalent p
raseodymium. Gated holes were observed in absorption lines to the two
lowest components of the D-1(2) manifold. At 1.4 K the gating ratio is
in excess of 1.5 x 10(4). Strong competition from the transient mecha
nism of optical pumping of hyperfine levels occurs below 6 K. (C) 1996
Optical Society of America