B. Delakowitz et al., A LITERATURE SURVEY OF MINERAL-SPECIFIC SORPTION DATA ON RADIONUCLIDES WITH RELEVANCE TO THE DISPOSAL OF RADIOACTIVE-WASTE, Journal of radioanalytical and nuclear chemistry, 213(2), 1996, pp. 109-125
A comparative review of mineral-specific: radionuclide sorption databa
ses created for performance assessment and reported in both the open l
iterature and ''grey literature'' (e.g. technical reports) has in part
shown poor quality of documentation describing the database selection
procedures. Inadequate information is available on the chemical speci
es of the radionuclide under consideration and the laboratory conditio
ns for determining Kd-values. Sorption data derived from literature ar
e neither comparable nor generally applicable due to the wide range in
the composition of the aqueous and the solid phases applied in migrat
ion experiments. Subsequently, standardized characterization and deter
mination procedures are needed. To improve the reliability of a mathem
atical model for the prediction of radionuclide sorption on cementitio
us and ash-type binder materials, determination of mineral-specific so
rption coefficients is indispensable.