FREQUENCY AND TIME-RESOLVED COHERENT STOKES RAMAN-SCATTERING IN CS2 USING INCOHERENT-LIGHT

Citation
Mj. Stimson et al., FREQUENCY AND TIME-RESOLVED COHERENT STOKES RAMAN-SCATTERING IN CS2 USING INCOHERENT-LIGHT, Chemical physics letters, 263(1-2), 1996, pp. 185-190
Citations number
10
Categorie Soggetti
Physics, Atomic, Molecular & Chemical
Journal title
ISSN journal
00092614
Volume
263
Issue
1-2
Year of publication
1996
Pages
185 - 190
Database
ISI
SICI code
0009-2614(1996)263:1-2<185:FATCSR>2.0.ZU;2-4
Abstract
A frequency and time resolved coherent Stokes Raman scattering signal from CS2(l) using noisy light (I-(2) CSRS) is presented. A broad range of frequencies are simultaneously sampled at each interferometric del ay, allowing acquisition times that are at least two orders of magnitu de shorter than previous single frequency detected interferometry expe riments. Sub-picosecond time resolution of radiation/matter beats call ed Rabi detuning oscillations is achieved by controlling the relative delay between twin nanosecond broadband pulses.