Magnetic Compton scattering, which measures solely the electron spin m
oment, has been used to provide direct evidence for the low value of t
he 4f moment on cerium in the ferrimagnetic compound CeFe2. The measur
ements were performed by using monochromatic, 61.34 keV photons with a
high degree of circular polarization produced by an elliptical multip
ole wiggler at the Accumulation Ring Source, KEK, Japan, Analysis of t
he Compton profile shows the 4f spin moment to be antiparallel to the
moment on Fe, This is consistent with the 4f moment as deduced from ne
utron-diffraction data yet conflicts markedly with the moment predicte
d in a series of nb initio band calculations, being less than half the
calculated value of 0.42 mu(B).