Ekf. Dang et Rj. Gooding, EFFECTS OF LONG-RANGED INTERACTIONS ON THE NUCLEATION DYNAMICS IN A PHI(6) MODEL, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics, 54(2), 1996, pp. 1383-1389
It is known that long-ranged interactions can play an important role i
n determining the dynamics of nudeation at a first-order phase transit
ion. For example, in a recent Letter by the present authors [Phys. Rev
. Lett. 74, 3848 (1995)] it was shown that during the annealing of an
amorphous thin film, long-ranged interactions generated by strains due
to elastic misfits could be responsible for the system becoming trapp
ed in a metastable secondary crystalline phase. In this paper we consi
der these long-ranged interactions in a more general context wherein o
nly symmetry considerations are invoked to determine if a particular i
nteraction potential is allowed. Their effects on a first-order phase
transition, as described by a single-component scalar phi(6) model, ar
e examined. These transitions are studied by means of Langevin simulat
ions. We find, through the evaluation of the time evolution of the ord
er parameter, the morphology of the steady state, and the time-depende
nt structure factor, that the precise form of the long-ranged interact
ion has a strong influence on the nature of nucleation dynamics, as we
ll as on the steady-state profiles.