CONSEQUENCES OF KINETIC INHOMOGENEITIES IN GLASSES

Citation
Dn. Perera et P. Harrowell, CONSEQUENCES OF KINETIC INHOMOGENEITIES IN GLASSES, Physical review. E, Statistical physics, plasmas, fluids, and related interdisciplinary topics, 54(2), 1996, pp. 1652-1662
Citations number
54
Categorie Soggetti
Physycs, Mathematical","Phsycs, Fluid & Plasmas
ISSN journal
1063651X
Volume
54
Issue
2
Year of publication
1996
Pages
1652 - 1662
Database
ISI
SICI code
1063-651X(1996)54:2<1652:COKIIG>2.0.ZU;2-7
Abstract
Many of the physical pictures used to rationalize the phenomenology of glassy dynamics rest upon a consideration of spatial fluctuations in the relaxation kinetics of the glass-forming liquid. We examine the wi re ranging consequences which flow from assuming the existence of tran sient kinetic inhomogeneities. These consequences include: strong and fragile behavior, two-step relaxation processes, nonlinear relaxation following temperature jumps, spatially correlated kinetics and non-Gau ssian behavior of incoherent processes. These general predictions are explored in simulations in which relaxation is governed by diffusing d efects.